Ubiquitous nature of multimode vibrational resonances in positron-molecule annihilation.
نویسندگان
چکیده
Positron annihilation on many molecules occurs via positron capture into vibrational Feshbach resonances, with annihilation rates often further enhanced by energy transfer to vibrational excitations weakly coupled to the positron continuum. Data presented here uncover another scenario in which the positron couples directly to a quasicontinuum of multimode vibrational states. A model that assumes excitation and escape from a statistically complete ensemble of multimode vibrations is presented that reproduces key features of the data.
منابع مشابه
Role of vibrational dynamics in resonant positron annihilation on molecules.
Vibrational Feshbach resonances are dominant features of positron annihilation for incident positron energies in the range of the molecular vibrations. Studies in relatively small molecules are described that elucidate the role of intramolecular vibrational energy redistribution into near-resonant multimode states, and the subsequent coupling of these modes to the positron continuum, in suppres...
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ورودعنوان ژورنال:
- Physical review letters
دوره 108 9 شماره
صفحات -
تاریخ انتشار 2012